1. She looked down at me with the bun of hair which was loose on her neck.
2. She looked down at me, and the bun of hair was loose on her neck.
Which is correct? Thanks in advance.
Only #2. #1 sounds like the bun helped her to look.
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An alternate version uses a small clause (a type of non-finite clause).
She looked down at me, the bun of hair loose on her neck.
CJ