The writer is present these things as facts, not possibilities.
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park sang joonlaughing though his mouth was filled with the blood of his body, and as he died, he would pronouncethough = as though = as if
park sang joonlaughing though his mouth was filled with the blood of his bodyIt is difficult to laugh when your mouth is filled with blood. "though" as a conjunction makes that point. "Although" could be used as well.
park sang joonbut his brother didn't die then.Maybe, but the description is about the death of the other brothers.
park sang joon"ashe diedFrom the time he started to die until he died. "As" means "during the time"