I could not access to the login of this account.
Is this right way to tell my concern?
You do not access "to" something, you just access it. If you remove the word "to" then your sentence would be grammatical, but normally you would just say "I could not log in to this account". g.
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You do not access "to" something, you just access it. If you remove the word "to" then your sentence would be grammatical, but normally you would just say "I could not log in to this account". "I could not access the login" sounds as if you are trying to say something different from this, e.g. you could not reach the login page at all. Is that what you mean?
I could not access the login page of this website.
I was not able to login to my account.